Review
Lanthanum-Based Perovskites for Catalytic Oxygen Evolution Reaction
Dr. Jeferson A. Dias,
Dr. Marcos A. S. Andrade Jr,
Hugo L. S. Santos,
Prof. Dr. Márcio R. Morelli,
Prof. Dr. Lucia H. Mascaro,
Dr. Jeferson A. Dias
Departamento de Engenharia de Materiais, Laboratório de Formulação e Sínteses Cerâmicas-LAFSCer, Universidade Federal de São Carlos, Rod. Washington Luís, km 235, São Carlos/SP, Brazil, 13565-905
Search for more papers by this authorCorresponding Author
Dr. Marcos A. S. Andrade Jr
Departamento de Química, Centro de Caracterização de Materiais Funcionais-CDMF-LIEC, Universidade Federal de São Carlos, Rod. Washington Luís, km 235, São Carlos/SP, Brazil, 13565-905
Search for more papers by this authorHugo L. S. Santos
Departamento de Química, Centro de Caracterização de Materiais Funcionais-CDMF-LIEC, Universidade Federal de São Carlos, Rod. Washington Luís, km 235, São Carlos/SP, Brazil, 13565-905
Search for more papers by this authorProf. Dr. Márcio R. Morelli
Departamento de Engenharia de Materiais, Laboratório de Formulação e Sínteses Cerâmicas-LAFSCer, Universidade Federal de São Carlos, Rod. Washington Luís, km 235, São Carlos/SP, Brazil, 13565-905
Search for more papers by this authorCorresponding Author
Prof. Dr. Lucia H. Mascaro
Departamento de Química, Centro de Caracterização de Materiais Funcionais-CDMF-LIEC, Universidade Federal de São Carlos, Rod. Washington Luís, km 235, São Carlos/SP, Brazil, 13565-905
Search for more papers by this authorDr. Jeferson A. Dias,
Dr. Marcos A. S. Andrade Jr,
Hugo L. S. Santos,
Prof. Dr. Márcio R. Morelli,
Prof. Dr. Lucia H. Mascaro,
Dr. Jeferson A. Dias
Departamento de Engenharia de Materiais, Laboratório de Formulação e Sínteses Cerâmicas-LAFSCer, Universidade Federal de São Carlos, Rod. Washington Luís, km 235, São Carlos/SP, Brazil, 13565-905
Search for more papers by this authorCorresponding Author
Dr. Marcos A. S. Andrade Jr
Departamento de Química, Centro de Caracterização de Materiais Funcionais-CDMF-LIEC, Universidade Federal de São Carlos, Rod. Washington Luís, km 235, São Carlos/SP, Brazil, 13565-905
Search for more papers by this authorHugo L. S. Santos
Departamento de Química, Centro de Caracterização de Materiais Funcionais-CDMF-LIEC, Universidade Federal de São Carlos, Rod. Washington Luís, km 235, São Carlos/SP, Brazil, 13565-905
Search for more papers by this authorProf. Dr. Márcio R. Morelli
Departamento de Engenharia de Materiais, Laboratório de Formulação e Sínteses Cerâmicas-LAFSCer, Universidade Federal de São Carlos, Rod. Washington Luís, km 235, São Carlos/SP, Brazil, 13565-905
Search for more papers by this authorCorresponding Author
Prof. Dr. Lucia H. Mascaro
Departamento de Química, Centro de Caracterização de Materiais Funcionais-CDMF-LIEC, Universidade Federal de São Carlos, Rod. Washington Luís, km 235, São Carlos/SP, Brazil, 13565-905
Search for more papers by this authorGraphical Abstract
Perovskite exploration: This Review provides a summary of the main results of lanthanum-based perovskites applied as electrocatalysts for the oxygen evolution reaction (OER). Beyond that, the main influence of A and B site substitutions, structural defects creation, structural distortions, material morphologies, the presence of supports, and orbital occupancy configurations on the perovskites’ OER catalytic activity are discussed in detail.
Abstract
Lanthanum-based perovskites have been gaining attention in recent years as cost-attractive and efficient catalysts for the oxygen evolution reaction (OER). Showing a simplified LaBO3 stoichiometry (B=transition metal cation), the structure and composition of the perovskites play key roles in their electrocatalytic performance. This paper aims to review the physicochemical concepts, structures, and recent advances on kinetic parameters for lanthanum-based perovskites for catalytic OER. First, advances on mechanisms and descriptors that govern general perovskites will be discussed in detail. Next, the current results for lanthanum cobaltite (LaCoO3), nickelate (LaNiO3), ferrite (LaFeO3), manganite (LaMnO3), and their derivations will be provided. Moreover, the existing results on less explored lanthanum perovskites for catalytic OER (LaCrO3, LaCuO3, LaVO3, and LaTiO3) will be also presented. The impacts of structural defects, orbital occupancy, materials morphology, and composition on the perovskite electrocatalytic performance will be assessed for each case. Finally, emerging trends for lanthanum-based perovskites will be provided.
Conflict of interest
The authors declare no conflict of interest.
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